添加链接
link管理
链接快照平台
  • 输入网页链接,自动生成快照
  • 标签化管理网页链接
多种同位素分析

Abstract:

This paper introduces several important theoretical and methodological issues involved with the strontium isotope archaeological research. The first is the variation pattern of strontium isotope ratios in the lithosphere and its influence on the study about human migration. Secondly, four restrictions of the strontium isotope method are addressed, the diagenetic contamination of bone and dentin samples, the overlapping effect of strontium isotope in different regions, the mixed effect of strontium isotope in teeth and bones, and the inability to identify migrant descendants. Finally, two major difficulties in the application of strontium isotope to the study of human migration are investigated. One is how to distinguish the migrant population in a site or cemetery, and the other is how to find the origin of the migrant population.

Key words: Strontium isotope, Human migration, Limitation, Multi-isotope analysis Kennedy B P, Folt C L, Blum J D, et al. Natural isotope markers in salmon[J]. Nature, 1997, 387(6635): 766-767 doi: 10.1038/42835 Bentley RA. Strontium isotopes from the earth to the archaeological skeleton: a review[J]. Journal of Archaeological Method & Theory, 2006, 13: 135-187 Faure G, Powell JL. Strontium Isotope Geology[M]. New York: Springer-Verlag, 1972 Faure G. Principles of isotope geology[M]. New York: Wiley, 1977 Faure G, Mensing T.M. Isotopes: principles and applications[M]. Hoboken: Wiley, 2005 Capo RC, Stewart BW, Chadwick OA. Strontium isotopes as tracers of ecosystems processes: theory and methods[J]. Geoderma, 1998, 82(1-3): 197-225 doi: 10.1016/S0016-7061(97)00102-X Blum JD, Taliaferro EH, Holmes WRT. Changes in Sr/Ca, Ba/Ca and 87Sr/86Sr ratios between trophic levels in two forest ecosystems in the northeastern U.S.A.[J]. Biogeochemistry, 2000, 49(1): 87-101 doi: 10.1023/A:1006390707989 Price TD, Burton JH, Bentley RA. The characterization of biologically available strontium isotope ratios for the study of prehistoric migration[J]. Archaeometry, 2002, 44(1): 117-135 doi: 10.1111/1475-4754.00047 Beard BL, Johnson CM. Strontium isotope composition of skeletal material can determine the birth place and geographic mobility of humans and animals[J]. Journal of Forensic Sciences, 2000, 45(5): 1049-1061 pmid: 11005180 Probst A, El Gh’mari A, Aubert D, et al. Strontium as a tracer of weathering processes in a silicate catchment polluted by acid atmospheric inputs, (Strengbach, France)[J]. Chemical Geology, 2000, 170: 203-219 doi: 10.1016/S0009-2541(99)00248-X Chadwick OA, Derry LA, Vitousek PM, et al. Changing sources of nutrients during four million years of ecosystem development[J]. Nature, 1999, 397: 491-497 doi: 10.1038/17276 Gallet S, Jahn BM, Lanoe BV, et al. Loess geochemistry and its implications for particle origin and composition of the upper continental crust[J]. Earth and Planetary Science Letters, 1998, 156: 157-172 doi: 10.1016/S0012-821X(97)00218-5 Whipkey CE, Capo RC, et al. The importance of sea spray to the cation budget of a coastal Hawaiian soil: A strontium isotope approach[J]. Chemical Geology, 2000, 168: 37-48 doi: 10.1016/S0009-2541(00)00187-X Price TD, Knipper C, Grupe G, et al. Strontium isotopes and prehistoric human migration: the Bell Beaker Period in central Europe[J]. European Journal of Archaeology, 2004, 7(1): 9-40 doi: 10.1177/1461957104047992 王兵, 李心清, 周会. 河流锶元素及其同位素地球化学研究现状与问题[J]. 地球与环境, 2009, 37(2): 170-177 Hoogewerff J, Papesch W, Kralik M, et al. The last domicile of the iceman from Hauslabjoch: A geochemical approach using Sr, C and O isotopes and trace element signatures[J]. Journal of Archaeological Science, 2001, 28(9): 983-989 doi: 10.1006/jasc.2001.0659 罗超, 郑洪波, 吴卫华, 等. 长江河水 87 Sr/ 86 Sr值的季节性变化及其指示意义:以长江大通站为例[J]. 地球科学进展, 2014, 29(7): 835-843 Wei G, Ma J, Liu Y, et al. Seasonal changes in the radiogenic and stable strontium isotopic composition of Xijiang River water: Implications for chemical weathering[J]. Chemical Geology, 2013, 343: 67-75 doi: 10.1016/j.chemgeo.2013.02.004 Bickle MJ, Bunbury J, Chapman HJ, et al. Fluxes of Sr into the headwaters of the Ganges[J]. Geochimica et Cosmochimica Acta, 2003, 67(14): 2567-2584 doi: 10.1016/S0016-7037(03)00029-2 Beard BL, Johnson CM. Strontium isotope compositions of skeletal material can determine the birth place and geographic mobility of animals and humans[J]. Journal of Forensic Science, 2000, 45(5): 1049-1061 Slovak NM, Paytan A. Applications of Sr Isotopes in Archaeology[M]. Handbook of Environmental Isotope Geochemistry. 2012: 743-768 Price TD, Blitz J, Burton JH, et al. Diagenesis in prehistoric bone: problems and solutions[J]. Journal of Archaeological Science, 1992, 19(5): 513-529 doi: 10.1016/0305-4403(92)90026-Y Koch PL, Tuross N, Fogel M. The effects of sample treatment and diagenesis on the isotopic integrity of carbonate in biogenic hydroxylapatite[J]. Journal of Archaeological Science, 1997, 24(5): 417-429 doi: 10.1006/jasc.1996.0126 Budd P, Montgomery J, Barreiro B, et al. Differential diagenesis of strontium in archaeological human dental tissues[J]. Applied Geochemistry, 2000, 15(5): 687-694 doi: 10.1016/S0883-2927(99)00069-4 Hillson S. Teeth[M]. Cambridge: Cambridge Univeristy Press, 2005 Sillen A. Biogenic and diagenic Sr/Ca in plio-pleistocene fossils of the Omo Shungura formation[J]. Paleobiology, 1986, 12(3): 311-323 doi: 10.1017/S0094837300013816 Sillen A, Sealy JC. Diagenesis of strontium in fossil bone: a reconsideration of Nelsonet al. (1986)[J]. Journal of Archaeological Science, 1995, 22(2): 313-320 doi: 10.1006/jasc.1995.0033 Kohn MJ, Schoninger MJ, Barker WW. Altered states: effects of diagenesis on fossil tooth chemistry[J]. Geochimica et Cosmochimica Acta, 1999, 63(18): 2737-2747 doi: 10.1016/S0016-7037(99)00208-2 Hoppe KA, Koch PL, Furutani TT. Assessing the preservation of biogenic strontium in fossil bones and tooth enamel[J]. International Journal of Osteoarchaeology, 2003, 13(1-2): 20-28 doi: 10.1002/oa.663 胡耀武, 王昌燧, 何德亮, 等. 古代人骨羟磷灰石的去污染研究[J]. 考古, 2006(7): 68-74 Snoeck C, Lee-Thorp J, Schulting R, et al. Calcined bone provides a reliable substrate for strontium isotope ratios as shown by an enrichment experiment[J]. Rapid Communications in Mass Spectrometry, 2015, 29: 107-114 doi: 10.1002/rcm.7078 Smith TM, Austin C, Green DR, et al. Wintertime stress, nursing, and lead exposure in Neanderthal children[J]. Science Advances, 2018, 4(10): eaau9483 doi: 10.1126/sciadv.aau9483 Grimstead DN, Clark AE, Rezac A. Uranium and Vanadium Concentrations as a Trace Element Method for Identifying Diagenetically Altered Bone in the Inorganic Phase[J]. Journal of Archaeological Method & Theory, 2017, 25: 689-704 孙继敏. 中国黄土的物质来源及其粉尘的产生机制与搬运过程[J]. 第四纪研究, 2003, 24(2): 175-183 赵春燕, 袁靖, 何驽. 山西省襄汾县陶寺遗址出土动物牙釉质的锶同位素比值分析[J]. 第四纪研究, 2011(1): 22-28 赵春燕, 胡松梅, 孙周勇, 等. 陕西石峁遗址后阳湾地点出土动物牙釉质的锶同位素比值分析[J]. 考古与文物, 2016(4): 128-133 陈骏, 仇纲, 杨杰东. 黄土碳酸盐Sr同位素组成与原生和次生碳酸盐识别[J]. 自然科学进展, 1997(6): 93-96 Currell MJ, Cartwright I. Major-ion chemistry, δ 13 C and 87 Sr/ 86 Sr as indicators of hydrochemical evolution and sources of salinity in groundwater in the Yuncheng basin, China[J]. Hydrogeology Journal, 2011, 19(4): 835-850 doi: 10.1007/s10040-011-0721-6 赵春燕, 李志鹏, 袁靖. 河南省安阳市殷墟遗址出土马与猪牙釉质的锶同位素比值分析[J]. 南方文物, 2015(3): 77-80+112 吴晓桐, 张兴香, 宋艳波, 等. 丁公遗址水生动物资源域的锶同位素研究[J]. 考古, 2018(1): 111-118 房书玉. 焦家遗址人口迁徙的锶同位素研究[D]. 济南: 山东大学, 2018 浙江省文物考古研究所, 嘉兴博物馆. 马家浜[M]. 北京: 文物出版社, 2019: 263-264 吴晓桐. 龙山时期黄河流域的人群迁移与资源流通[D]. 合肥: 中国科学技术大学, 2018 Lugli F, Cipriani A, Arnaud J, et al. Suspected limited mobility of a middle Pleistocene woman from southern Italy: strontium isotopes of a human deciduous tooth[J]. Scientific Reports, 2017, 7: 8615 doi: 10.1038/s41598-017-09007-5 石玉秀. 组织学与胚胎学(第3版)[M]. 北京: 高等教育出版社, 2018 Scharlotta I, Goriunova OI, Weber A. Micro-sampling of human bones for mobility studies: diagenetic impacts and potentials for elemental and isotopic research[J]. Journal of Archaeological Science, 2013, 40(12): 4509-4527 doi: 10.1016/j.jas.2013.07.014 尹若春, 张居中, 杨晓勇. 贾湖史前人类迁移行为的初步研究——锶同位素分析技术在考古学中的运用[J]. 第四纪研究, 2008, 28(1): 50-57 赵春燕, 杨杰, 袁靖, 等. 河南省偃师市二里头遗址出土部分动物牙釉质的锶同位素比值分析[J]. 中国科学(地球科学), 2012, 42(7): 1011-1017 Ezzo JA, Johnson CM, Price TD. Analytical perspectives on prehistoric migration: a case study from east-central Arizona[J]. Journal of Archaeological Science, 1997, 24(5): 447-466 doi: 10.1006/jasc.1996.0129 Pirce TD, Arcini C, Custin I, et al. Isotopes and human burials at Viking Age Birka and the Mälaren region, east central Sweden[J]. Journal of Anthropological archaeology, 2018, 49: 19-38 doi: 10.1016/j.jaa.2017.10.002 Price TD, Nakamura S, Suzuki S, et al. New isotope data on Maya mobility and enclaves at classic Copan, Honduras[J]. Journal of Anthropological Archaeology, 2014, 36: 32-47 doi: 10.1016/j.jaa.2014.02.003 Wright LE. Identifying immigrants to Tikal, Guatemala: defining local variability in strontium isotope ratios of human tooth enamel[J]. Journal of Archaeological Science, 2005, 32(4): 555-566 doi: 10.1016/j.jas.2004.11.011 Fenner JN, Wright LE. Revisiting the strontium contribution of sea salt in the human diet[J]. Journal of Archaeological Science, 2014, 44: 99-103 doi: 10.1016/j.jas.2014.01.020 Slovak NM, Paytan A, Wiegand BA. Reconstructing middle horizon mobility patterns on the coast of Peru through strontium isotope analysis[J]. Journal of Archaeological Science, 2009, 36(1): 157-165 doi: 10.1016/j.jas.2008.08.004 Giblin JI. Strontium isotope analysis of Neolithic and copper age populations on the great Hungarian plain[J]. Journal of Archaeological Science, 2009, 36(2): 491-497 doi: 10.1016/j.jas.2008.09.034 Zhang XX, Burton JH, Jin ZY, et al. Isotope studies of human remains from Mayutian, Yunnan province, China[J]. Journal of Archaeological Science, 2014, 50: 414-419 doi: 10.1016/j.jas.2014.08.001 赵春燕, 王明辉, 叶茂林. 青海喇家遗址人类遗骸的锶同位素比值分析[J]. 人类学学报, 2016, 35(2): 212-222 陈曦. 梁带村芮国墓地出土西周时期人骨的骨化学特征研究[D]. 西安: 西北大学, 2012 赵春燕, 何驽. 陶寺遗址中晚期出土部分人类牙釉质的锶同位素比值分析[J]. 第四纪研究, 2014, 34(1): 66-72 中国社会科学院考古研究所. 二里头(1999- 2006)[M]. 北京: 文物出版社, 2014: 1288-1294 山西省考古研究所, 运城市文物工作站, 芮城县旅游文物局, 等. 清凉寺史前墓地[M]. 北京: 文物出版社, 2016: 538-543 Hodell DA, Quinn RL, Brenner M. Spatial variation of strontium isotopes ( 87 Sr/ 86 Sr) in the Maya region: a tool for tracking ancient human migration[J]. Journal of Archaeological Science, 2004, 31(5): 585-601 doi: 10.1016/j.jas.2003.10.009 Bentley RA, Knipper C. Geographical patterns in biologically available strontium, carbon and oxygen isotope signatures in prehistoric SW Germany[J]. Archaeometry, 2005, 47(3): 629-644 doi: 10.1111/j.1475-4754.2005.00223.x Thomsen E, Andreasen R. Agricultural lime disturbs natural strontium isotope variations: implications for provenance and migration studies[J]. Science advances, 2019, 5(3): eaav8083 doi: 10.1126/sciadv.aav8083 Evans JA, Montgomery J, Wildman G. Spatial variations in biosphere 87 Sr/ 86 Sr in Britain[J]. Geological Society of London, 2010, 167(1): 1-4 Willmes M, Bataille CP, James HF, et al. Mapping of bioavailable strontium isotope ratios in France for archaeological provenance studies[J]. Applied Geochemistry, 2018, 90: 75-86 doi: 10.1016/j.apgeochem.2017.12.025 Hartman G, Richards M. Mapping and defining sources of variability in bioavailable strontium isotope ratios in the eastern Mediterranean[J]. Geochimica Et Cosmochimica Acta, 2014, 126: 250-264 doi: 10.1016/j.gca.2013.11.015 Laffoon JE, Davies GR, Hoogland ML. Spatial variation of biologically available strontium isotopes ( 87 Sr/ 86 Sr) in an archipelagic setting: a case study from the Caribbean[J]. Journal of Archaeological Science, 2012, 39(7): 2371-2384 doi: 10.1016/j.jas.2012.02.002 Wang XY, Tang ZH. The first large-scale bioavailable Sr isotope map of China and its implication for provenance studies[J]. Earth-Science Review, 2020, 210: 1-21 Wang XY, Tang ZH, Dong XX. Distribution of strontium isotopes in river waters across the Tarim basin: a map for migration studies[J]. Journal of the Geological Society, 2018, 175 (6): 967-973 doi: 10.1144/jgs2018-074 White CD, Spence MW, Stuart-Williams HLQ. Oxygen isotopes and the identification of geographical origins: the valley of Oaxaca versus the valley of Mexico[J]. Journal of Archaeological Science, 1998, 25(7): 643-655 doi: 10.1006/jasc.1997.0259 Wu XT, Hein A, Zhang XX, et al. Resettlement strategies and Han imperial expansion into southwest china: a multimethod approach to colonialism and migration[J]. Archaeological and Anthropological Sciences, 2019, 11: 6783 doi: 10.1007/s12520-019-00949-7 张兴香, 李雍, 吴晓桐, 等. 黄河流域出土龙山时期扬子鳄骨板的多种同位素研究[J]. 人类学学报, 2019, 38e: 313-324 Hu Y. Thirty-Four Years of Stable Isotopic Analyses of Ancient Skeletons in China: an Overview, Progress and Prospects[J]. Archaeometry, 2018, 60(1): 144-156 doi: 10.1111/arcm.12367 Li W, Zhou L, Lin Y, et al. Interdisciplinary study on dietary complexity in Central China during the Longshan Period (4.5-3.8 kaBP): New isotopic evidence from Wadian and Haojiatai, Henan Province[J]. The Holocene, 2021, 31(2): 258-270 doi: 10.1177/0959683620970252 Samuelsen JR, Potra A. Biologically available Pb: A method for ancient human sourcing using Pb isotopes from prehistoric animal tooth enamel[J]. Journal of Archaeological Science, 2020, 115: 1-23